Gonna make this easy for the person below me: Pokémon X/Y.
The franchise's first foray into 3D was also the one they put the most effort in. They made over 700 Pokémon models just for this one little 3DS games, along with all their animations and redone cries, even adding special cry variations and animations for the Pokémon-Amie minigame (not the best thing ever made, but a rare attempt to actually have a connection with your Pokémon outside of just battling). Now we live in an age where Game Freak tells us how impossible it would be to have every Pokémon in the HD games, despite them reusing the same models and animations that were made for X/Y twelve years ago.
X/Y also had the best soundtrack hands down. All the battle themes are iconic, and some of the other music stands out a lot too like most of the route themes, the Pokémon League theme, and the end credits. The story has its critics and understandably so, but beneath its cringy exterior I think there's something really genuine in it, and as Masuda's last game as director, I really feel like there was some heart put into it.
Lastly Kalos was just the nicest-looking region and had the best roster of Pokémon. It was a small roster yeah, but it gave me many of my favorites like Greninja, Gogoat, Pangoro, Aegislash, and a lot of other cool ones.