Gears, all of them.

Maybe some rpg's from the 5th and 6th generations.

I would buy them 200 for collection ! in order :

Langrisser 1-5
Shining Force 1-3
Valkyria chronicle 1-3
Mass effect 1-3 (never played them, sigh at me)

1) fallout3/new Vegas collection (ps3)
2)onimusha (ps2)
3) Resident Evil zero
4)resident evil outbreak file #1 #2
5) Tomb raider 1-3

Lost Odyssey and All the main Onimusha games.

Skyrim does sound like a good candidate. Never played it.
Half life collection just before HL3.
GTA from 3 to 4, all 4 console games remake, not just ports.

Kotor
Crash Bandicoot (all ps1 games)
Wipeout Fusion
Super Mario 64 (on a home console this time please)
Mario Party 1-3 (mainly 2/3 but they'd have to shove 1 in I guess)

Red dead redemption, uncharted collection, infamous collection, okami, vanquish and dbz burst limit.

Twilight Princess HD

Darkcloud
Legend of Legaia