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For me:

N64 - Super Mario 64, Super Smash Bros., Castlevania, Banjo-Kazooie, Conker's Bad Fur Day, Mario Kart 64
Wii U - Super Mario 3D World, Splatoon, New Super Mario Bros. U, New Super Luigi Bros. U, Super Smash Bros., Mario Kart 8.

I don't know, I think it's a tie. Even if I think the Wii U games are superior, the N64 ones are very memorable for me.