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As a system? Well the Wii had the ability to function as a Gamecube as well, so I'd say the Wii is better.

Games-wise? Depends on how you look at it. Mainline Mario games were better on the Wii, 3rd party offerings were much much much better on the Gamecube. Pokemon was better on the Gamecube, Pikmin was better on the Wii.

They're both my favourite home consoles, so personally it's a tie.