Im surprised that more discussion about the games that are on the Virtual Console doesnt happen here.
What with 250 games available, there must be a very decent selection of games besides the requisite Zeldas, Sonics, and Marios that go unnoticed.
Personally, I only own two games on VC and both are great games.
Landstalker (genesis) - an isometric adventure game that has a personality and style which make up for its sometimes frustrating camera position.
Streets of Rage 2 - a classic beat-em up which i bought despite having the original cartridge. This is a very accessible game, with an arcade feel. I really recommend this to everybody that even remotely enjoys the genre.
What games have you found that are worth considering?