I dont use Crunchyroll but....
For the top 5 I would recommend....
-Mobile Suit Gundam (original from 1979) - then Zeta Gundam and I would go to Char's Counterattack movie in that order (Skip ZZ)
-Clannad
-ERASED
-Fullmetal Alchemist: Brotherhood
-Higurashi: When They Cry
Some of my most favorite anime include that I would recommend to anyone (these are all scored 10 via my MAL account)
TV
-Attack on Titan (all seasons)
-Bakemonogatari/Nisemonogatari/Owarimonogatari
-Beastars (Both seasons, final season coming soon)
-Black Clover
-Blue Gender
-Blue Lock (best sports anime, second season in the future)
-Chainsaw Man
-Clannad (Both seasons - the extras/specials can be skipped)
-Code Geass: Lelouch of the Rebellion (all seasons)
-Death Note
-Deca-Dence
-Demon Slayer: Kimetsu no Yaiba (all seasons and movies)
-Detective Conan (all of the main anime, specials, OVAs, and movies - especially the movies, they are top tier lol)
-Dragon Ball/Z/GT/Super (All movies too)
-Durarara (All seasons)
-Edens Zero (2nd season starting soon)
-ERASED
-Fate/stay night
-Fate/Zero (both seasons)
-Fate/Apocrypha
-Fire Force (Both seasons, 3rd season on its way)
-Fullmetal Alchemist: Brotherhood
-Gleipnir
-Goblin Slayer (and the movie)
-Hi Score Girl (All seasons and specials)
-Higurashi: When They Cry (all seasons)
-Jujutsu Kaisen
-Komi Can't Communicate (both seasons)
-Little Witch Academia
-Lupin III (Original from 1971)
-Mob Psycho 100 (All seasons)
-Mobile Suit Gundam (original from 1979)
-Mobile Suit Zeta Gundam
-Mobile Suit Gundam: The 08th MS Team
-Mobile Suit Gundam 0083: Stardust Memory
-Mobile Suit Victory Gundam
-Mobile Suit Gundam Wing
-Mobile Suit Gundam 00 (both seasons - movie can be skipped)
-Mobile Fighter G Gundam
-My Dress-Up Darling (Second season soon)
-My Hero Academia (All seasons, specials and movies)
-Naruto/Naruto Shippuden
-Neon Genesis Evangelion
-Now and Then, Here and There
-Odd Taxi
-One Punch Man (All seasons)
-Radiant (Both seasons)
-Ranking of Kings
-Raven of the Inner Palace
-Remake Our Life!
-Sonny Boy (highly recommend)
-Spice and Wolf (all of the seasons and specials/OVAs)
-Spy x Family (all of it)
-The Faraway Paladin (Second season soon)
-The Rising of the Shield Hero (The first season imo was the only good one)
-To Your Eternity (Both seasons)
-Trigun (original)
-Tsuki ga Kirei
-Umineko: When They Cry
-Yu Yu Hakusho: Ghost Files (though I recommend stop watching after the Dark Tournament lol)
OVA
-FLCL
Movie
-Castle in the Sky
-From Up on Poppy Hill
-Kiki's Delivery Service
-My Neighbor Totoro
-Princess Mononoke
-Spirited Away
-The Secret World of Arrietty
-The Girl Who Leapt Through Time
-When Marnie Was There
-Whisper of the Heart
Non-Japanese animations I highly recommend
-Fairies Albums - All seasons (Chinese)
-Link Click - second season starting soon (Chinese)
-Scissor Seven - all seasons (Chinese)
-The Daily Life of the Immortal King - All seasons (Chinese)
-The Dining of Link Lee - both seasons (Chinese)
-The God of High School (Korean)
-Tower of God (Korean)
