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SNES to N64 is a pretty obvious choice. Nintendo also was much more successful moving Mario and Zelda into 3-D where series like Mega Man, Castlevania, Contra, Street Fighter, and Mortal Kombat crashed into the polygon ceiling,

I'm also going to say 3DS to Switch was a pretty huge leap, not just graphically but for the "switching" ability.

Gamecube looked like a real improvement over N64 as well, and I think that gets understated. GC is what I'd wished PS2 looked like.