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My favorite video game track of all time is Sky Sanctuary Zone from Sonic & Knuckles.

http://youtube.com/watch?v=oNXBpzDp1K8

However... there is one song that may steal my heart. The more I listen to it, the more amazing it becomes... Gusty Garden Galaxy from Super Mario Galaxy

http://youtube.com/watch?v=A0R6FnpqylE

Other Notables...

Metropolis Zone (Sonic 2)
http://youtube.com/watch?v=yRuJfhEeCe8

Rattle Battle (DKC2)
http://youtube.com/watch?v=vT9w3zk5vsc

Skytown (Metroid Prime 3)
http://youtube.com/watch?v=7P7jdnU06ew

Opening (The Legend of Zelda: Wind Waker)
http://youtube.com/watch?v=zJCsOte2bcw

Metal Gear Solid 4 Love Theme (SSBB)
http://youtube.com/watch?v=uUfKFElJ9sA