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Definitely comes down to either Mario 64, Wii Sports, or BotW.

All three of those were hugely popular and fantastically fun games that were the peak of mega system sellers. And all three felt like something completely new - Mario 64 for just being the first legendary 3D game on consoles and moving the biggest gaming mascot into 3D incredibly well, Wii Sports for showing off a whole new way to play games and was endlessly fun especially with friends/family, BotW because it gave players open world freedom unmatched by any other game before and resurrected the greatness of the iconic Zelda franchise which had got quite stale in the previous two entries.

SMB, Tetris, and SMW all get honorable mention for being fantastic games and system sellers but I just feel they aren't on the level of those other three, although SMW comes very close and could arguably be added to the first list.