I just completed RE4 on PSVR2 last night, while great, it's not in my top 10. Top 40 maybe after a second play through. Both RE8 and RE7 are better games in VR.
It's a shame Civilization didn't make it in, would have had my vote.
Or Everquest which is my personal nr 1.
I voted for The Last of Us for this decade, yet plenty games go in front for the GoaT.
BotW is in my top 10 yet preceded by Wind Waker which is not in the poll.
I'll cop out and vote for the game that started it all, Pong.
(It's just gonna be a battle between OoT and BotW anyway :p)