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On a technical level, TLOU. It wasn't my favorite game either graphically or as a game, though. Personally I'd give it to Ni no Kuni for being a playable Ghibli film.

Best on Wii is definitely SMG.

360, dunno. I was pretty much done with 360 after 2009, and the best looking games I saw on it by that point were Soulcalibur IV and Tales of Vesperia, and ToV, while having nice, colorful cel-shaded graphics, was not in the same league as Halo or Gears.