Very tough question.
I'd say Super Mario Bros 3. It totally changed up the formula, expanded in huge ways and has been influential for decades to come and pushed the NES to it's limits. Super Mario World is probably the better game, but not nearly as influential, hence why SMB3 wins this one.
The Nintendo eShop rating Thread: http://gamrconnect.vgchartz.com/thread.php?id=237454 List as Google Doc: https://docs.google.com/spreadsheets/d/1aW2hXQT1TheElVS7z-F3pP-7nbqdrDqWNTxl6JoJWBY/edit?usp=sharing
The Steam/GOG key gifting thread: https://gamrconnect.vgchartz.com/thread/242024/the-steamgog-key-gifting-thread/1/
Free Pc Games thread: https://gamrconnect.vgchartz.com/thread/248138/free-pc-games/1/