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Lynels are the coolest ones, and the hardest ones to fight, I am now powerful enough to soundly beat red and blue ones, but the white and silver ones are still difficult. The silver ones can do every move in the book, even teleport. Didn't even try the hard mode yet so I can only imagine the golden lynels.

Guardians are probably the most intimidating ones, and equally difficult when aren't equipped for them yet. They can make a total mess of things. It's also the only enemy I'm afraid to lose my Hylian Shield to because a direct hit of it's laser does like a billion damage. They're great to fight though and you feel like a bad-ass beating one if them.

I like both those more than the ones with health bars, and they're tougher too. Talusses are just annoying most times and Hinox are cool, but not that hard even early on unless one of them corners you. Molduga are cool, and can be a bit difficult until you figure out a few tricks and safe spots.

I pick Lynels. Closely followed by the Guardians.