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1. Smeagol/Gollum from "Lord of the Rings" always felt sad seeing the corruption of the one ring eventually consume him. The multiple personality scenes showed the internal struggle and made me feel bad even if he tried to stop the heroes.

2. Koba from "Dawn of the Planet of the Apes" was handled well by keeping him for two films to allow you to see his understandable prejudice against humans and how it was inevitable his differences with Caesar would end one of them.