Vita / 3ds for sure, some of the best games you can find.
Mobile phone... eerrr not so much, there is some good games on them but unless it's something slow and turn based like Alphabears then I feel like you are constantly fighting the lack of any actual controls, I've sadly played a lot more Snake on my old Nokia 5110 than I have played any game on my Xperia... when it comes to best mobile gaming device I've used which is also a phone (a fucking terrible phone) the N-Gage at least had button controls (no L+R tho) but yeah N-Gage was a very capable 100mhz gaming machine.
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