Mummelmann said:
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Not at home atm so here is just the ones i can recall right now that i currently am using/testing:
Deadly Dragons/Deadly Monsters: http://www.nexusmods.com/skyrim/mods/3829/?
Enemy Ai overhaul: http://www.nexusmods.com/skyrim/mods/40491/? not sure how good it will hold up further on as one advances up the levels though
I also use mods that while not cranking up difficulty on their own add mnore creatures and npc patrols, mainly the mods Immersive Patrols and Immersive Creatures.
while not using it myself i hear the skyrim Redone mod also can make combat more difficult since it rebalances weapons and armors