Xbox vs GC .. Which had best looking games? Would love an outside perspective

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Both can do things the other can't.

GC couldn't do the extensive per-pixel lighting and normal mapping of games like Splinter Cell Chaos Theory and Chronicles of Riddick.

Xbox couldn't do the amount of polygons and effects that Rogue Squadron 2 and 3 pushed while running at 60fps.

It all depends on which approach looks more visually appealing to the individual.