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Easily Iron Man for me; its Hollywood adaptation was actually entertaining with Captain America coming in second. Iron Man 2 was brutal to watch, if you know its back story. They could have chosen a better villain, with a better plot. I expected more from Thor, and I do not know if Marvel even know what they are doing with Hulk.
Also, in my honest opinion, involving the character in the end credits of The Avengers would only complicate things further. I am not confident Marvel and/or Hollywood can make a decent transition happen. I predict an X3 breakdown.