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1 The World Ends With You The best rpg of the geration and easily one of the best of all time.
2 999: 9 Hours. 9 Persons, 9 Doors The best visual novel game ever, so many plot twists in the end that will make your brain explode.
3 Radiant Historia Time Travel + Great story + Nice Battle System = Incredible Game
4 Elite Beat Agents Addictive music game that will test your might with the stylus
5 Castlevania Order of Eclesia A tough as nails action game that is worthy of the castlevania brand
6 Pokemon Black/White New pokemon and an impressive online structure make this one of the best pokemon games to be released on a handled.
7 Shin Megami Tensei Devil Survivor The best strategy game on the DS with a tough difficulty and great story with multiple endings.
8 Okamiden Not only has the best 3d graphics for the ds, it is also its best adventure game.
9 Call of Duty Black Ops The best shooter on the ds complete with a lengthy campaign, online and even the zombies mode with more maps than its console counterparts.
10 Chrono Trigger The best game of all time ported to our loved handled. It could easily be #1, but its a port so other ds games need more spotlight.

Honorable Mentions: Rune Factory, The Last Window The Secret of Cape West, Bleach Dark Souls, Trauma Center, Dragon Quest 9, Super Robot Taisen, Ghost Trick, Super Scribblenauts, Professor Layton, FF4, Sonic Colours.... I could keep going but lets leave it at that =).