Definitely agree about Command & Conquer.
Seems like EA tried to fix something that wasn't really broken with the ye old "drugs and shit-flinging" - method. It didn't work.
Other series that haven't been mentioned:
Jagged Alliance
X-Com
Earthworm Jim
Icewind Dale (well, kinda - I'm not a big fan of the series, but if one wants something to showcase D&D 4 in a video game...)
Psychonauts
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