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1. Goldeneye 64 (The game just made you want to keep playing)
2. Half-Life 1 (Great games that really have spawned many others CS,TFC,DoD)
3. Half-Life 2 (Built off of a successful game in Half-Life and made for a great game).
4. Halo 1 (Really brought what a lot of better PC shooters had at the time).
5. Perfect Dark 64 (Not as much fun as Goldeneye, but it was pretty close still a wonderful game. That pushed the N64's limits).