Any of the touch generation games - Brain Training, NSMB, Mario Kart, Nintendogs, Pokemon... can't go wrong. Cooking Mama is ok, but not the same league as the others.
Mario Party DS rocks as well. Elite Beat if they like music.
PS - I can't recommend "No More Heroes" to be honest - its a very flawed, frustrating experience - with smatterings of coolness. Much better Wii titles out there.
Gesta Non Verba
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