1. Chrono Crusade
2. Bleach
3. Naruto
4. Devil May Cry
5. Trigun
6. Trinity Blood
7. Saiyuki
8. Samurai X
9. Kenshin
10. Full Metal Alchemist

I would put Last Order - Final Fantasy VII #1 if you can count that being an actual Anime, i love it more than all of Chrono Crusade, but i listed anime's with more than one episode.

Ok I'd say :

12 pts - Now and Then, Here And There
11 pts - Grave of the Fireflies
10 pts - Maison Ikkoku
09 pts - Omoide Poro Poro (Only Yesterday)
08 pts - The two Rurouni Kenshin OVA
07 pts - Mononoke Hime
06 pts - Gunslinger Girls
05 pts - Perfect Blue
04 pts - Azumanga Daioh
03 pts - Tokyo Godfathers
02 pts - Kaze no Tani no Nausicaä (Nausicaä of the Valley of the Wind)
01 pts - Evangelion

Okay, I took FOREVER to telly all the votes, I didn't add some because people give some like 12 points? Whaaat?

Naruto: 26 points
FullMetal Alchemist: 23 points
Dragon Ball Z: 21 point
Evangelion: 20 points
Gundam - 17 points
Bleach: 16 points
Cowboy Bebop: 16 points
Yu Yu Hakusho - 15 point
Elfen Lied - 13 points
Ninja Scoll movie – 10 points
Kenshin – 10 points
Pokemon – 10 points
Ranma 1/2 - 9 points
Princess Mononoke- 8 points
Escaflowne – 8 points
Hellsing OVA - 7 points
Last Exile - 5 points
One Piece – 5 points
Galaxy Express 999 – 5 points
Gantz – 5 points
Nausicaa - 4 points
golden boy: 4 points
Robotech – 4 points
grave of the fireflies- 4 points
Innocent Venus - 4 points
Club to Death Angel – 4 points
FLCL – 4 points
Macross - 4 points
.hack//SIGN - 3
GunGrave - 3 points
Digimon -3
Martian Successor Nadesico - 3 Points
The Melancholy of Haruhi Suzumiya - 3 points
Fruits Basket – 3 points
Sakura Card captor – 3 points
Dr. Slump – 3 points
Tnjou Tenge - 2 points
Air Gear - 2 points
Please Teacher – 7 points
Paranoid Agent - 2 Points
Onegai Twins – 2 points
My Neighbour Totoro – 2 points
Monster - 2 points
his and her circumstance- 1 point
Diamond Dust Drops - 1 point
Go Lion - 1 Point
Saint Seiya - 1 point
Shaman King – 1 point
Record of Lodos Wars – 1 point
Doraemon -1 point
Planetes – 1 point
Trigun – 1 point
Ghost in a Shell – 1 point