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PS2 for me. As others have mentioned, the sheer variety and quantity of interesting titles is hard to overlook. PS2 also represents, for me, the best intersection of great Sony-produced games and great third-party games. Sony's output was a bit wobbly during the PS1 era but really hit its stride across the sixth gen. In my mind, the PS2 is the only Sony home console where you could argue the best part of its library consisted of first-party productions -- either designed or published in house. 

1. Ico
2. Metal Gear Solid 3
3. Shadow of the Colossus
4. Devil May Cry
5. Jak and Daxter: The Precursor Legacy