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Well, it's easy to say the series peaked with CoD4: Modern Warfare, because that was the last game they truly made an effort to innovate, and every game since has just been an annual re-package/re-skin with minimal improvements, and almost all of those 'improvements' derived from modern trends.

That being said, my favourite before I stopped playing CoD for good was BlOps. Modern Wafare 2 was just a more refined version of CoD 4. World at War actually took some steps back with it's multiplayer, but brought in Zombie mode. BlOps felt like it had the best mix of everything-- Zombie mode, weapons, multiplayer game modes etc.

The games after that aren't even worth mentioning.