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Not sure if I can think of a top 5 but my personal favs in no order:
Ansem - First KH only, great voice acting and very simple easy premise.
Reapers - Proof that AI still technically isn't free thinking. A great version of AI though, love me some AI characters.
Kefka - Dude said he's destroy the world. He did.
Handsome Jack - He was the hero... stupid Vault Hunters. (not sure how they are going to top him in Borderlands 3)
Captain Walker - You know the guy, the one you play as in Spec Ops.... those who haven't played this game, play it.





Hmm, pie.