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That's a tough one as many games in the Wii excelled in one wah but fell short in another. Xenoblade is the most obvious, with massive and fairly lush environments realized beautifully and the LOD being impressively detailed. But all things were a bit fuzzy up close and character models were sixth gen level.

If I had to pick one..........
Mario Galaxy 1 or 2 would be one possibility. Metroid Prime 3 and other M also deliver though.

But honestly? I love the graphics of The Legend of Zelda: Skyward Sword.