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AZWification said:

You should definitely try Half-Life 2 and BioShock! Trust me, you won't regret it!

Agreed.

IkePoR, if you're looking for atmospheric, deliberate first-person shooters with good stories, look no further than these two. Half-Life 2, especially, is brilliant in the way it tells its story indirectly. Much like Retro with Metroid Prime, the developers at Valve "show, don't tell" their story in Half-Life 2.

Some other great single-player campaings can be found in Halo: Combat Evolved, Half-Life, Red Faction, Medal of Honor (which you mentioned), F.E.A.R., GoldenEye 007, Perfect Dark, Star Wars: Republic Commando, Unreal, Call of Duty, and the original Killzone.