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While the DS had a lot of great games, the PSP had an overall better quality library. Even when you compare genres that the Nintendo DS excelled at, the PSP titles are just as good if not better at times.

Nintendo has a decent amount of good platformer titles, 2D and 3D, but so does the PSP. Castlevania Dracula X Chronicles, Prinny, Prinny 2, Mega Man Maverick Hunter X, Gurumin, Tomb Raider Legend, Tomb Raider Anniversary, etc.

When it comes to just about every genre that the DS doesn't excel at quite as well as the PSP, then it's no contest. RPG, Shooter, Shmup, Fighting, Action/Adventure, etc.

The only games that the DS has that the PSP can't "touch(pun intended") are touch screen type casual games. Rarely are they any good, but there's the rare title like Feel the Magic Xx/Xy and Rub Rabbits which are very good.