All time would be Street Fighter 2. It improved greatly over its predecessor and revolutionized gaming forever.
The rest:
Assassin's Creed 2
Infamous 2
Uncharted 2
FInal Fantasy IX (Though not really a sequel to anything)
Prototype 2
Battle Arena Toshinden 2
Tekken 3
Tekken 5: Dark Resurrection
I'll add more later.
I am the Playstation Avenger.
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