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Turkish said:
There can only be 2 answers:

Shadow of the Colossus
Journey

This. And the music for Ico is very well chosen too. It works so well in Ico since the music keeps it distance most of the time which makes it all the more effective. The problem with most games is that you get tired of the music long before the game is over, not in these 3.

I would add Pixeljunk 4AM too, although it's debatable if that's a game.

The last stage of Pixeljunk sidescroller also stands out for me, perfect marriage between music and on screen action.