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Wii: Super Smash Brothers-Only beats Mario because of its never ending appeal for multiplayer.
360: Orange Box-Kind of cheating, but Half-Life 2 is awesome, and so are the rest of the games included.
GC: Super Smash Brothers-Again, multiplayer fun never ends. Resident Evil 4 is a close second.
N64: Legend of Zelda: Ocarina of Time-The greatest game of all time.
SNES: Chrono Trigger-Best RPG ever made, with lots of replay value due to the many endings. Super Mario Allstars would be my second choice, with 4 games in 1 (5 if you get the version with Super Mario World!).