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1)

  • God of War III
  • Ratchet & Clank: Tools of Destruction
  • Rathcet & Clank: A Crack in Time
  • Batman: Arkham Asylum
  • Bioshock
  • Vanquish
  • Super Street Fighter IV
  • Red Dead Redemption
  • Mass Effect 2
  • If you have a buddy to play split-screen Mercenaries with, Resident Evil 5. If not... Marvel vs. Capcom 3?

(I'm not sure if Bioshock, Vanquish SSFIV, RDR and ME2 are better than the 360 versions, but if your taste is anything like mine, they're must-haves anyway.)

2) Castle Crashers, Fat Princess, Mega Man 9 & 10, and... Uh... Some PS1 stuff?

3) I hardly ever play online, but I haven't had any such problems.