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Kain.

No other character has made me feel such a plethora of emotions in a game. I thought he best carried the overlying theme throughout the game. He was in a constant struggle with trying to redeem himself.

From his unique ability; his jealousy; his struggle with selflessness; and his eventual redemption he was the focus of many plot twists throughout the game and was perhaps the most pivotal character.

I think he's easily the most interesting character in the series.

Commonman makes a pretty solid case for Rydia too.