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While the N64's AAA games are better, the sheer volume of solid A and AA ps1 games makes it very close.

N64- Mario 64, Banjo and Kazooie 1 and 2, Conkers, Jet Force Gemini, OOT and Majoras Mask, 007, Perfect Dark, Turok 1 and 2, Smash Bros., Wave race, F-Zero, S. Mario Kart, 1080, Star Fox, Killer Instinct, Paper Mario…

PS1- Wipeout 1- 3, Crash Bandicoots 1-3, FF7, FF8, FF9, Parasite Eve, Vandal Hearts, Castlevania SOTN and Chronicles, Fear Effect 1 and 2, Silent Hill, RE 1-3, Dino Crisis, Heart of Darkness, Odd World 1 and 2, Doom and Final Doom, Legacy of Kain, Soul Reaver, Tomb Raider 1 and 2, Ape Escape, Bloody Roar, Jumping Flash, Medievil 1 and 2, Metal Gear Solid, Twisted Metal, R-types and delta, N2O, Nanotech Warrior, Einhander, Warhawk, etc….

Looking at the above lists I can safely conclude that if you owned only one of these systems than you missed out! By the way forgive me if I missed ur favorite. Also, at the time N64 was defiantly my favorite so....