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The Ghost of RubangB said:
Anything from Gainax.

They did Neon Genesis Evangelion, which starts out normal and gets weirder every episode and has the weirdest ending of any anime. But for the purposes of this thread I'll recommend FLCL, and Magical Shopping Arcade Abenobashi, which are 2 of the weirdest anime I've seen in my life. And they switch genres several times per episode. FLCL is only 6 episodes and is really really good and everybody should see it.

And Paranoia Agent by Satoshi Kon. It's only 13 episodes, and has my favorite intro and outro of any animated series.

Paranoia Agent and Eva are awful but Abenobashi is awesome.