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for me
1. Valkyria Chronicles
2. Disgaea 3
3. LBP
4. Warhawk
5. Yakuza 3
6. Lumines Supernova
7. Heavenly Sword
8. Ratchet & Clank Future: Tools of Destruction
9. Eye of Judgment
10. ---
MGS 4 - soon will be on 360,
Echochrome - already is on psp,
PixelJunk Monsters - soon will be on psp in enchanced edition,

i didn't mention:
Resistance series - those are average shooters so it's only a must have if you want to play only exclusive games, are a FPS fan and bought every other exclusive fps on ps3. besides there are similar games on 360.
Killzone 2 - same as Resistance series, it's a must only for graphical whores who like brown-green-greyish realistic style graphics,
Uncharted series same as Killzone 2.
MLB Show - well besides americans and some japanese baseball fans who really give a damn about baseball? not to mention that nobody outside of baseball fans know the rules of this game.
Ridge Racer 7 - although i'm a big fan of RR games - it's hard to call it exclusive now since it's basically the same game as RR6 with some additional tweaks here and there.
Flower - i mean come on who would buy a console for that thing? if you're putting this on the list than everyone can put My Aquarium(if i remember correctly the name) on the wii on must have lists,
Folklore - it's an average game - although a good one, but still a long way till anyone would call it a must have.
Buzz and Singstar - 360 have the same games in its onw versions(Lips and Scene It or somethin) so it's hard to call must have exclusives.