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The Anarchyz said:
Graphics: N64 had a better 3D engine and memory expansion, PS1 only was slightly better in 2D (although, not near the Saturn)
Cutscenes: PS1 because it had the FMVs
Controller: N64 had an awesome controller, PS1 at first didn't bring anything new, then the Dual-Analog came, and then the Dualshock, my favorite because it merged the SNES layout (best ever) and N64 analog-rumble in one controller.
Sound: PS1 hands down, better chip and more formats, also more space for CD-quality sound.
Storage: Obviously PS1, low space cartridges vs CDs.
Delay: Obviously N64, almost electronic speed vs CD-reading speed.

Games: Let me see:

N64: The Legend of Zelda: Ocarina of Time (best of the system IMO), Super Mario 64, Goldeneye 007, Mario Kart 64, Super Smash Bros, Pokemon Stadium, Majora's Mask, Perfect Dark, the Mario Parties, Paper Mario, Superman 64 (just kidding jejeje)...

PS1: Final Fantasy VIII-VII-IX!!!, Xenogears, Parasite Eve, Megaman 8-X4-X5-X6-Legends I-II, Chrono Cross, the Crashes and the Spyros, Gran Turismo, Wipeout, Suikoden, the Breath of Fire's, Dragon Quest VII, Star Ocean 2, Tales of Destiny-Eternia, Resident Evil 1-2-3, Tenchu, the fighting games that weren't on the Saturn (like the Tekken's), Final Fantasy Tactics, Tony Hawk series, Legend of Mana, Metal Gear Solid, Silent Hill, Persona 1-2...

I have to go with PS1, but i still love both consoles...

 

forgot about Crash, Twisted Metal, Spyro, Tomb raider, Medal of Honor and Driver ;)