I am playing my first ever Assassins Creed game (Black Flag) on PS3 and it is so technically impressive, suddenly the Naughty Dog games dont seem special anymore. They really figured out the PS3 at the end of its lifecycle. The joke about waiting till they unleash the true power of PS3 is invalid! I was already impressed what Ubisoft did with Driver San Francisco, it was so smooth and good looking compared to other racing games on PS3, but Black Flag is yet on another level, it is like Unsharted three fold.
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Deus Ex (2000) - a game that pushes the boundaries of what the video game medium is capable of to a degree unmatched to this very day.