unfortunately I don't know a trilogy that I feel is deserving of this honor..
LotR - (I'm a big fan of the books) doesn't do it for me in movie 2+3, in the big battles there is just sth feeling off imo
Back to the Future - consistently good-very good, but individually the movies aren't up there
Toy Story - same as above, I was really surprised how genuinely entertaining the third one was considering how stupid Shrek and Ice Age became the more movies they put out for those, yet not enough overall
original Star Wars trilogy - looking back they've lost too much of their fascination to me
new Star Wars trilogy - lol, no
Batman - I've yet to watch TDKR, but TDK already was a step down from Batman Begins imo, so I don't expect it to turn that around tbh
Matrix - no
Godfather - 1 and 2 are excellent, but I've yet to watch the 3rd one as most people rate that one a few steps below the first 2
I think TV shows just do a better job at maintaining a consistenly superb quality while telling a longer story.
edit:
I guess I misread the question a bit, so just as conclusion movies probably Toy Story 3 and Back to the Future 3 tied for the top