Smash Bros. runs impressively for Wii U hardware, but it's visuals range from decent to highly unimpressive.
Wind Waker HD is beautiful, and it's a great remaster of the Gamecube's best looking game.
But Rayman Legends... Omg, it's basically flawless. It gets my vote, though I prefer playing it on PS4/PS3 and Vita. Regardless of platform, everyone who cares about video games needs to play it.