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I'm not much of a soundtrack listener nowadays, but one film soundtrack I enjoyed was the Underworld: Evolution soundtrack. That one holds a special place in my heart for having 2 original songs sung by 2 of my favorite vocalists kicking off the album as well as a third written specifically for the film (that chorus, man):

I also really liked the Queen of the Damned soundtrack for the 5 original songs from Jonathan Davis (surely you're familiar with those) that couldn't make it onto the album for contractual reasons (his versions, anyway) despite being featured in the film:

The rest of the soundtrack ain't too shabby, either.